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Recognizing its causal power, contemporary scholars of media effects commonly leverage experimental methodology. For most of the 20th century, however, political scientists and communication scholars relied on observational data, particularly after the development of scientific survey methodology around the mid-point of the century. As the millennium approached, Iyengar and Kinder’s seminal News That Matters experiments ushered in an era of renewed interest in experimental methods. Political communication scholars have been particularly reliant on experiments, due to their advantages over observational studies in identifying media effects. Although what is meant by “media effects” has not always been clear or undisputed, scholars generally agree that the news media influences mass opinion and behavior through its agenda-setting, framing, and priming powers. Scholars have adopted techniques and practices for gauging the particular effects these powers have, including measuring the mediating role of affect (or emotion). Although experiments provide researchers with causal leverage, political communication scholars must consider challenges endemic to media-effects studies, including problems related to selective exposure. Various efforts to determine if selective exposure occurs and if it has consequences have come to different conclusions. The origin of conflicting conclusions can be traced back to the different methodological choices scholars have made. Achieving experimental realism has been a particularly difficult challenge for selective exposure experiments. Nonetheless, there are steps media-effects scholars can take to bolster causal arguments in an era of high media choice. While the advent of social media has brought new challenges for media-effects experimentalists, there are new opportunities in the form of objective measures of media exposure and effects.